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A prodigious contributor to the Hebrew press, his column in the American Hebrew weekly Hadoar dealt with political and, especially with literary events. From 1907 Scharfstein also published educational texts embracing Hebrew literature, Jewish education, Bible, and Hebrew language.
His historical works as a Jewish educator include Ha-Heder be-Hayyei Ammenu (1943) and Toledot ha-Hinnukh be-Yisrael ba-Dorot ha-Aharonim (5 vols., 1960–66); and his autobiographical works comprise Arba'im Shanah ba-Amerikah (1955–56). Among his contributions to Hebrew lexicography is Ozar ha-Ra'yonot va-ha-Pitgamim (3 vols., 1966). From 1940 Scharfstein was editor of the educational periodical Shevilei ha-Hinnukh.